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On-line SPICE-SPIN+X Seminars

On-line Seminar: 25.11.2020 - 15:00 (CET)

Three-dimensional magnetic systems: the future is bright!

Claire Donnelly, University of Cambridge

Three dimensional magnetic systems promise significant opportunities for applications, for example providing higher density devices and new functionalities associated with complex topology and greater degrees of freedom [1,2]. With recent advances in both characterization and nanofabrication techniques, the experimental investigation of these complex systems is now possible, opening the door to the elucidation of new properties and rich physics.
For the characterization of 3D nanomagnetic systems, we have developed techniques to map both the three-dimensional magnetic structure, and its response to external excitations. In a first demonstration of X-ray magnetic nanotomography [3,4], we determined the complex magnetic structure within the bulk of a μm-sized soft magnetic pillar. The magnetic configuration contained vortices and antivortices, as well as Bloch point singularities [3]. With these new datasets comes a new challenge concerning the identification of such nanoscale topological objects within complex reconstructed magnetic configurations. To address this, we have recently implemented calculations of the magnetic vorticity [5,6], that make possible the location and identification of 3D magnetic solitons, leading to the first observation of nanoscale magnetic vortex rings [6].
In addition to the static magnetic structure, the dynamic response of the 3D magnetic configuration to excitations is key to our understanding of both fundamental physics, and applications. With our recent development of X-ray magnetic laminography [7,8], it is now possible to determine the magnetisation dynamics of a three-dimensional magnetic system [7].
Finally, recent advances in nanofabrication make possible the fabrication of complex 3D magnetic nanostructures [9], leading to the realisation of artificial chiral structures [10] and 3D spintronic devices [11]. These new experimental capabilities for 3D magnetic systems open the door to complex three-dimensional magnetic structures, and their dynamic behaviour.

PDF file of the talk available here

[1] Fernández-Pacheco et al., “Three-dimensional nanomagnetism” Nat. Comm. 8, 15756 (2017)
[2] Donnelly and V. Scagnoli, “Imaging three-dimensional magnetic systems with X-rays” J. Phys. D: Cond. Matt. (2019).
[3] Donnelly et al., “Three-dimensional magnetization structures revealed with X-ray vector nanotomography” Nature 547, 328 (2017).
[4] Donnelly et al., “Tomographic reconstruction of a three-dimensional magnetization vector field” New Journal of Physics 20, 083009 (2018).
[5] Cooper, “Propagating magnetic vortex rings in ferromagnets.” PRL. 82, 1554 (1999).
[6] Donnelly et al., “Experimental observation of vortex rings in a bulk magnet” Nat. Phys. (2020)
[7] Donnelly et al., “Time-resolved imaging of three-dimensional nanoscale magnetization dynamics”, Nature Nanotechnology 15, 356 (2020).
[8] Witte, et al., “From 2D STXM to 3D Imaging: Soft X-ray Laminography of Thin Specimens”, Nano Lett. 20, 1305 (2020).
[9] Skoric et al., “Layer-by-Layer Growth of Complex-Shaped Three-Dimensional Nanostructures with Focused Electron Beams” Nano Lett. 20, 184 (2020).
[10] Sanz-Hernández et al., “Artificial Double-Helix for Geometrical Control of Magnetic Chirality” ACS Nano 14, 8084 (2020).
[11] Meng et al., “Non-planar geometrical effects on the magnetoelectrical signal in a three-dimensional nanomagnetic circuit” In preparation.

Resonant p-wave oscillations of Josephson current in Nb-Bi2Te2.3Se0.7-Nb topological junctions

Alexander Golubov

Recent proposals of inducing p-wave superconductivity by sandwiching a conventional s- wave superconductor (S) with a topological insulator (TI) triggered a burst of research activity. Topological superconductors harness the inherent electron – hole symmetry of excitations in a superconductor with the helical nature of the electronic states in topological materials, that may lead to Majorana zero energy states. Various theoretical models focused on possible pairing symmetries of the proximity induced superconducting order in topological layers. Several experimental groups already realized S-TI interfaces and S-TI-S junctions, and studied the Josephson current across them. Few papers have reported unusual Shapiro steps consistent with the formation of the p-wave correlations. However, measurements that could provide the definitive evidence of the p-wave superconductivity should be phase-sensitive, to discriminate between the p- and other (s-, d-...) pairings symmetries.
In this work we report a new type of oscillations of the critical Josephson current in magnetic field observed in the Nb-Bi2Te2.3Se0.7-Nb junctions [1,2]. The ultra-short period ∼ 1 Oe of these oscillations and their sharply peaked shape reflect the resonant transmission via Andreev bound states with the ultra-fine ∼ 1 μeV interlevel spacing. We argue that the ultra- fine oscillations revealed in our S-TI-S devices is the direct consequence of the p-wave superconducting order induced at S-TI contacts.

[1] V.S. Stolyarov, D.S. Yakovlev, S.N. Kozlov, O.V. Skryabina, D.S. Lvov, A.I. Gumarov, O.V. Emelyanova, P.S. Dzhumaev, I.V. Shchetinin, R.A. Hovhannisyan, S.V. Egorov, A.M. Kokotin, W.V. Pogosov, V.V. Ryazanov, M.Yu. Kupriyanov, A.A. Golubov, D. Roditchev. COMMUNICATIONS MATERIALS 1:38 (2020)| https://doi.org/10.1038/s43246-020-0037-y | www.nature.com/commsmat.
[2] V.S. Stolyarov, D. Roditchev, V.L Gurtovoy, S.N. Kozlov, D.S. Yakovlev, O.V. Skryabina, V.M. Vinokur, A.A. Golubov, submitted to Nature Physics.

Flat Bands in Flatlands

Jeanie Lau

In a flat band system, the charge carriers’ energy-momentum relation is very weakly dispersive. The resultant large density of states and the dominance of Coulomb potential energy relative to the kinetic energy often favor the formation of strongly correlated electron states, such as ferromagnetism, nematicity, antiferromagnetism, superconductivity, and charge density waves. The advent of two-dimensional (2D) materials and their heterostructures has ushered in a new era for exploring, tuning and engineering of flat band system. Here I will present our results on transport measurements of high quality few-layer 2D material devices, including intrinsic magnetism and helical edge states in few-layer graphene, and observation of both superconductivity and the Mott-like insulating state in a tBLG device with a twist angle of ~0.93°.

Long range unconventional Josephson effect across a half metallic ferromagnet

Jacobo Santamaria

The Josephson effect results from the coupling of two superconductors across a non- superconducting spacer to yield a quantum coherent state. In ferromagnets, singlet (opposite- spin) Cooper pairs decay over very short distances, and thus Josephson coupling requires a nanometric spacer. This is unless equal-spin triplet pairs are generated which, theoretically, can couple superconductors across much longer distances. Despite many experimental hints of triplet superconductivity, long range triplet Josephson effects have remained elusive. In this talk I will discuss a micron-range Josephson coupling across the half-metallic ferromagnet
La0.7Sr0.3MnO3 combined with the high-temperature superconductor YBa2Cu3O7 in planar junctions. These display the Josephson physics’ hallmarks: critical current oscillations due to flux quantization and quantum phase locking under microwave excitation. The marriage of high- temperature quantum coherent transport and full spin polarization brings unique opportunities for the practical realization of superconducting spintronics, and enables novel strategies for quantum computing.

Topological phases combining superconductivity and magnetism

Mario Cuoco

In this talk I will present different routes to generate and manipulate topological phases due to the interplay between superconductivity and magnetism. The search for new variants of semimetals (SMs) recently highlighted the interplay of Dirac fermions physics and magnetism. Indeed, antiferromagnetic (AFM) SMs can be obtained where both time and inversion are broken while their combination is kept [1,2] or due to chiral- [2] and time-symmetry [2,3] combined with non-symmorphic transformations [2]. Here, we discuss materials, i.e. transition metal oxide systems, that can exhibit AFM-SM phase due to orbitally directional double- exchange effects [4, 2]. In this context, the impact of s-wave spin-singlet pairing on AFM-SMs with Dirac points or nodal loops at the Fermi level [5] is generally shown to convert the semimetal into various types of nodal topological superconductors. The changeover from fully gapped to gapless phases is dictated by symmetry properties of the AFM-superconducting state that set out the occurrence of a large variety of electronic topological transitions [4].
Finally, I will focus on various quantum platforms marked by spin-singlet or spin-triplet pairing interfaced with non-trivial magnetic patterns and discuss the nature of the emerging topological phases [6,7,8]. The coexistence of ferromagnetism or antiferromagnetism with spin-triplet superconductivity is also analysed and discussed with respect to relevant materials cases.

[1] P. Tang, Q. Zhou, G. Xu, and S.-C. Zhang, Nat. Phys. 12, 1100 (2016).
[2] W. Brzezicki and M. Cuoco, Phys. Rev. B 95, 155108 (2017).
[3] S. M. Young and B. J. Wieder, Phys. Rev. Lett. 118, 186401 (2017).
[4] W. Brzezicki, C. Noce, A. Romano, and M. Cuoco, Phys. Rev. Lett. 114, 247002 (2015).
[5] W. Brzezicki and M. Cuoco, Phys. Rev. B 97, 064513 (2018).
[6] M. T. Mercaldo, M. Cuoco, P. Kotetes, Phys. Rev. B 94, 140503(R) (2016).
[7] A. Romano, P. Gentile, C. Noce, I. Vekhter, M. Cuoco, Phys. Rev. Lett. 110, 267002 (2013). 8. P. Kotetes, M. T. Mercaldo, M. Cuoco, Phys. Rev. Lett. 123, 126802 (2019).
[9] M. T. Mercaldo, P. Kotetes, M. Cuoco, Phys. Rev. B 100, 104519 (2019).

Geometrically driven effects in curved superconducting nanostructures

Paola Gentile

The most recent advances in nanotechnology have demonstrated the possibility to create flexible semiconductor nanomaterials which are bent into curved, deformable objects ranging from semiconductor nanotubes, to nanohelices, etc. The consequences of the nanowire bending on the electronic quantum properties have been demonstrated to become of particular importance in systems with structure inversion asymmetry, where the interplay between nanoscale deformations and Rashba spin-orbit coupling (RSOC) [1] allows an all-geometrical and electrical control of electronic spin textures and spin transport properties [2,3], including the possibility to induce topological nontrivial phases [4-6]. In the presence of superconducting pairing, inversion symmetry breaking (ISB) makes neither spin nor parity good quantum numbers anymore. The ensuing mixing of even spin-singlet and odd spin- triplet channels leads to a series of novel features, from unconventional surface states to topological phases. Within this framework, we have explored the impact that nanoscale geometry has on superconducting properties of low-dimensional materials, showing that the interplay between RSOC and shape deformations can lead to novel paths for a geometric manipulation of the superconducting state, both for spin-singlet and spin-triplet quantum configurations [7], then significantly affecting the Josephson effect of weak links between Rashba coupled straight superconducting nanowires with geometric misalignment [8] as well as between nanowires of topological superconductors with non-trivial geometric curvature [9].

[1] P. Gentile., M. Cuoco, C. Ortix, SPIN, Vol. 3, No. 2, 1340002 (2013).
[2] Z.-J. Ying, P. Gentile, C. Ortix, M. Cuoco, Phys. Rev. B 94, 081406(R) (2016).
[3] G. Francica, P. Gentile, M. Cuoco, EPL 127, 30001 (2019).
[4] P. Gentile, M. Cuoco, C. Ortix, Phys. Rev. Lett. 115, 256801 (2015).
[5] P. G., V. Benvenuto, C. Ortix, C. Noce, M. Cuoco, Condens. Matter 4 (1), 25 (2019).
[6] S. Pandey, N. Scopigno, P. Gentile, M. Cuoco, C. Ortix, Phys. Rev. B 97, 241103(R) (2018).
[7] Z.-J. Ying, M. Cuoco, C. Ortix, P. Gentile, Physical Review B 96, 100506(R) (2017).
[8] Z.-J. Ying, M. Cuoco, P. Gentile, C. Ortix, 2017 16th International Superconductive Electronics Conference (ISEC), IEEE Xplore (2018).
[9] G. Francica, M. Cuoco, P. Gentile, Phys. Rev. B 101, 094504 (2020).

Angle Bilayer Graphene – Superconductors, Orbital Magnets, Correlated States and beyond

Dimitri Efetov

When twisted close to a magic relative orientation angle near 1 degree, bilayer graphene has flat moire superlattice minibands that have emerged as a rich and highly tunable source of strong correlation physics, notably the appearance of superconductivity close to interaction-induced insulating states. Here we report on the fabrication of bilayer graphene devices with exceptionally uniform twist angles. We show that the reduction in twist angle disorder reveals insulating states at all integer occupancies of the four-fold spin/valley degenerate flat conduction and valence bands, i.e. at moire band filling factors nu = 0, +(-) 1, +(-) 2, +(-) 3, and reveals new superconductivity regions below critical temperatures as high as 3 K close to - 2 filling. In addition we find novel orbital magnetic states with non-zero Chern numbers. Our study shows that symmetry-broken states, interaction driven insulators, and superconducting domes are common across the entire moire flat bands, including near charge neutrality. We further will discuss recent experiments including screened interactions, fragile topology and the first applications of this amazing new materials platform.

Helium Ion Beam Modification of High Transition Temperature Superconductors

Shane Cybart

In Feynman’s infamous 1959 lecture entitled, "There's Plenty of Room at the Bottom " he inspired and foreshadowed the emergence of nanoengineering. He suggested that finely focused electron, and ion beams would aid our eyes and hands to precisely engineer structures at the atomic level. Currently, electron beam lithography systems and gallium focused ion beams are ubiquitous in nanotechnology and can routinely be used to create structures of the order of tens of nanometers. However, the ability to scale to the sub-10 nm has been a technological challenge until the development of gas field ion sources (GFIS) over the past decade. The GFIS source, utilizes a single crystal tungsten wire sharpened to just 3 atoms. Helium gas is field ionized by one of these atoms, creating a helium ion beam with diameter of only 0.25nm! This instrument is emerging as an important tool for sub-10nm structuring of materials. Helium ion beams have significant advantages. Helium is small and chemically inert which allows it to be used for direct modification of materials properties without etching away material or employing resists.
My research group has been utilizing GFIS for direct patterning of ceramic high-temperature superconducting materials for quantum electronics. The helium ion beam induces nanoscale disorder from irradiation into the crystalline structure which converts the electrical properties of the material from superconductor to insulator. Insulating feature sizes of less than 2nm have been successfully demonstrated and many unique novel devices have been realized. Much of this success is due to the irradiation sensitivity of electrical transport in high temperature superconductors. This sensitivity results from loosely bound oxygen atoms (~1-8ev) in the crystal lattice that are easily displaced into interstitial or anti-site defects. I will describe details of the GFIS materials modification process and highlight applications in quantum sensing, and high frequency detection.

Topological superconductivity in gold leads to Majorana Zero Mode Pair

Jagadeesh S. Moodera

Surfaces and interfaces play a pivotally defining role for many of the topologically driven nontrivial quantum phenomena. A good example is the prediction of Majorana zero modes (MZMs or the Majorana pair) to occur in a topological superconductor (TSC) – viz., superconducting surface state of gold. [1] A fermion in a TSC can separate in space into two parts known as MZMs. Thus, Majorana pair are Fermionic states, each of which is an antiparticle of itself, and are required to always appear in pair together with its partner. According to the theoretical proposal of Potter and Lee, [1] under the right conditions, a superconducting gold nanowire with (111) crystalline surface with its large Rashba spin-orbit (S-O) splitting could host the Majorana pair. Utilizing the interplay between superconductivity, S-O coupling and Zeeman field we laid the foundation to realize MZM. [2] We have experimentally optimized a novel stable heterostructures, to achieve all these three interactions, to directly observe the MZM pair using a low temperature with high vector field scanning tunneling microscope, by probing the ferromagnetic EuS island over the gold surface. [3] With this two-dimensional stable metal platform, by means of the Shockley surface state (SS) of (111)-gold (Au) with induced superconductivity, we can envision a novel approach to building non-local qubits that are intrinsically fault-tolerant. In this talk I will be presenting our path towards the observation of MZMs.
Supported by John Templeton Foundation Grants No. 39944 and 60148, ONR Grants N00014-16-1-2657, N00014-20-1-2306 and NSF DMR 1700137

[1] A. C. Potter & P. A. Lee PRL 105, 227003 (2010); PRB 85, 094516 (2012)
[2] Peng Wei, Sujit Manna, Marius Eich, Patrick Lee and J. S. Moodera, Phys. Rev. Lett. 122, 247002 (2019)
[3] Sujit Manna, Peng Wei, Yingming Xie, Kam Tuen Law, Patrick A. Lee and Jagadeesh S. Moodera, Proc. Natl. Acad. Sci. 117 (16) 8775-8782 (Apr. 21, 2020)

Topological superconductivity in a van der Waals heterostructure

Peter Liljeroth

There has been a surge of interest in designer materials that would realize electronic responses not found in naturally occurring materials. For example, it is not clear if topological superconductivity [1], which is a key ingredient in topological quantum computing, exist in any single material. These limitations can be overcome in designer van der Waals (vdW) heterostructures, where the desired physics emerges from the engineered interactions between the different components.
Molecular-beam epitaxy (MBE) growth allows the construction of vertical heterostructures with clean and high-quality interfaces [2]. We use MBE to grow islands of ferromagnetic CrBr3 [3] on a superconducting NbSe2 substrate. This combines out of plane ferromagnetism with Rashba spin-orbit interactions and s-wave superconductivity and allows us to realizate topological superconductivity in a van der Waals heterostructure [4]. We characterize the resulting one-dimensional edge modes using low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS). The use of vdW heterostructures with uniform and high-quality interfaces is promising for future device structures and further control of topological superconductivity through external stimuli (e.g. electrostatic gating).

[1] M. Sato, and Y. Ando, Topological superconductors: a review. Rep. Prog. Phys. 80, 076501 (2017)
[2] S. Kezilebieke, M. N. Huda, P. Dreher, I. Manninen, Y. Zhou, J. Sainio, R. Mansell, M.M. Ugeda, S. van Dijken, H.-P. Komsa, P. Liljeroth, Electronic and Magnetic Characterization of Epitaxial VSe2 Monolayers on Superconducting NbSe2, Commun. Phys. 3, 116 (2020)
[3] W. Chen, Z. Sun, Z. Wang, L. Gu, X. Xu, S. Wu, C. Gao, Direct observation of van der Waals stacking–dependent interlayer magnetism. Science 366, 983 (2019)
[4] S. Kezilebieke, M. N. Huda, V. Vaňo, M. Aapro, S.C. Ganguli, O.J. Silveira, S. Głodzik, A.S. Foster, T. Ojanen, P. Liljeroth, Topological superconductivity in a designer ferromagnet-superconductor van der Waals heterostructure, arXiv:2002.02141 (2020)