Orbital Hall Effect in 2D Materials

Tatiana G. Rappoport

The field of spintronics blossomed in the last decade, driven by the use of spin-orbit coupling to generate and manipulate spin currents in non-magnetic materials. In these systems, the efficient conversion between charge and spin currents is mediated by spin-orbit. Great progress in the manipulation of the orbital angular momentum of light has also been achieved in the last decades, leading to a large number of relevant applications. Still, electron orbitals in solids were less exploited, even though they are known to be essential in several underlying physical processes in material science. The orbital-Hall effect (OHE), similarly to the spin-Hall effect (SHE), refers to the creation of a transverse flow of orbital angular momentum that is induced by a longitudinally applied electric field. The OHE has been explored mostly in three dimensional metallic systems, where it can be quite strong. However, several of its features remain unexplored in two-dimensional (2D) materials.

We then investigate the OHE in multi-orbital 2D insulators, such as transition metal dichalcogenides. We show that the OHE in these systems is associated with exotic momentum-space orbital textures. This intrinsic property emerges from the interplay between orbital attributes and crystalline symmetries and does not rely on the spin-orbit coupling. Our results indicate that multi-orbital 2D materials can display robust OHE that may be used to generate orbital angular momentum accumulation, and produce strong orbital torques that are of great interest for developing novel spin-orbitronic devices.